English
聯系我們
網站地圖
郵箱
舊版回顧



蘇州納米所等在石墨烯氣凝膠領域取得進展

文章來源:蘇州納米技術與納米仿生研究所   發布時間:2019-05-10  【字號:     】  

  石墨烯氣凝膠,經由石墨烯片層三維搭接、組裝而來的石墨烯宏觀體材料,具有三維連續多孔網絡結構,表現出高比表面積、高孔隙率、優異導電性能及電化學行為,在能源存儲、傳感、吸附、復合材料等領域有重要應用前景。然而,目前常規石墨烯氣凝膠的三維組裝以石墨烯片層間的“面-面”局部搭接方式為主,進而形成具有三維無規連續多孔網絡。石墨烯片層間的這種“面-面”堆垛-搭接方式,是一種無規、隨機組裝,往往會使得部分石墨烯片層形成類石墨結構,造成石墨烯本征性能(如比表面積、力學、電學等)損失。此外,傳統石墨烯氣凝膠所具有的這種無規三維多孔網絡還引入高界面電阻及曲折離子通道問題,對電化學行為中的電荷-離子傳輸及有效電化學活性面積維持帶來負面影響,成為制約石墨烯材料在電化學能源器件中應用的瓶頸。因此,如何設計新的石墨烯組裝策略,制備高性能石墨烯氣凝膠材料,仍是一個重要挑戰。

  針對石墨烯氣凝膠目前存在的問題,中國科學院蘇州納米技術與納米仿生研究所研究員張學同領導的氣凝膠團隊通過“局部氧化刻蝕”在氧化石墨烯片層上進行造孔,獲得孔洞氧化石墨烯,隨后將孔洞氧化石墨烯與還原劑分散液高度濃縮,實現其液晶化,進一步經原位溶膠凝膠及超臨界干燥獲得各向異性“孔洞石墨烯”氣凝膠,如圖所示。所得各向異性“孔洞石墨烯”氣凝膠由孔洞石墨烯片層經有序排列而成,表現出規整的三維多孔網絡(規整的孔道/孔壁及孔壁上的大量微孔)、低密度(42-55 mg cm-3)、高導電性(~165 S m-1)、高比表面積(537~837 m2 g-1)等諸多優點。最后將該氣凝膠作為電極材料,輔以共晶混合物“水-甲酰胺”作為低溫電解液,構建出可在溫度低至零下40°C的環境中正常工作的柱狀低溫熱電化學池,表現出低離子傳輸阻力(15.7 Ω)及高輸出功率(3.6 W m-2)。當15個熱電化學池進行串聯組裝成器件時,可實現~2.1 V電壓的穩定輸出,在低溫能源器件應用中表現出重要應用前景。

  相關成果以High-Efficiency Cryo-Thermocells Assembled with Anisotropic Holey Graphene Aerogel Electrodes and a Eutectic Redox Electrolyte 為題發表在國際期刊《先進材料》(Advanced Materials20191901403)上。博士生李廣勇、碩士董大鵬及澳門大學教授洪果為論文共同第一作者,張學同與英國UCL教授宋文輝為論文共同通訊作者,合作者還包括中國科學技術大學教授閆立峰。論文工作獲得國家重點研發計劃、國家自然科學基金委、英國皇家學會-牛頓高級學者基金等資助。

  圖:各向異性“孔洞石墨烯”氣凝膠基本表征:氧化石墨烯片層的透射電鏡照片(a1)及氧化石墨烯液晶的偏光顯微鏡照片(b1),孔洞氧化石墨烯片層的透射電鏡照片(a2)及氧化石墨烯液晶的偏光顯微鏡照片(b2),氧化石墨烯及孔洞氧化石墨烯片層的拉曼光譜(c),各向異性“孔洞石墨烯”氣凝膠的光學照片(d)、掃描電鏡照片(ef)、力學(g)、電學(h)及比表面積數據(i)。




(責任編輯:葉瑞優)

附件:

專題推薦

相關新聞


© 1996 - 中國科學院 版權所有 京ICP備05002857號  京公網安備110402500047號  聯系我們

地址:北京市三里河路52號 郵編:100864

5号彩www.565hc.com www.978614.com | www.6595.xyz | www.156990.com | www.75xb.com | www.8ij.com | www.7665.cm | www.012244.com | www.41978.com | www.234222.cc | www.377072.com | www.382098.com | 620527.com | www.139653.com | www.028012.com | www.589346.com | www.193361.com | www.335726.com | 500彩票www.401280.com | www.tb21.com | 715915.com | www.931079.com | www.978914.com | www.298112.com | www.618628.cc | www.590531.com | www.720811.cc | www.885106.com | www.916412.com | 949306.com | www.oc70.com | 600万彩票www.549810.com | www.138421.com | www.263862.com | 085539.com--163a.com | 019013.com | www.85965.cc | www.10635.com | www.8564.vip | www.98uh.com | www.187696.com | www.6310.me | 969043.com | www.39778.cc | 862947.com | 437000.cc | www.79je.com | www.243327.com | www.60430.com | www.631686.com | www.291045.com | www.cp7198.com | 2321.biz | www.871787.com | www.w02.net | www.45qz.com | www.84xn.com | www.607.tv | 692307.com | www.ij38.com | 大赢家彩票平台www.223065.com | ui04.com | 杏彩www.00840m.com | www.uz4.com | www.043191.com | 713093.com | 855649.com | 478522.com | www.220451.com | 977808.com | www.2bc.cc | www.45421.com | www.s86.pw | www.785905.com | www.52il.com | www.785818.com | www.gh86.com | www.186739.com | www.689195.com | 50097.com | www.669251.com | www.846083.com | www.7049.cc | 乐彩网www.3416l.com | www.cai1477.com | www.55bd.com | www.2028.date | www.2203.me | www.266801.com | www.898082.com | www.701757.com | 大赢家彩票平台www.810706.com | www.oo36.com | www.060065.com | www.510855.com | www.348329.com | www.240360.com | 407448.com | www.qg94.com | www.317353.com | 902166.com | www.521450.com | www.735283.com | www.507873.com | 078035.com | www.620096.com | www.x17.cc | www.50538.com | www.420186.com | www.lq6.com | www.994424.com | www.789393.com | www.16500.com | www.912935.com | 500彩票www.50026k.com | 500彩票www.50074d.com | www.678022.com | www.44482.cc | www.60700.com | www.l89.club | www.ag21.com | www.694625.com | www.653751.com | www.348022.com | www.681897.com | www.974848.com | www.879993.com | www.qd18.com | 797057.com | www.947164.com | www.951705.com | www.183365.com | www.854496.com | www.800717.com | www.pn.com | www.737931.com | www.594939.com | 582242.com | 佰萬彩票www.560529.com | 彩掌柜www.czg1.com | 500彩票www.364877.com | 712566.com | 257281.com | www.588667.com | www.721058.com | www.706663.com | 714583.com | www.750330.com | www.85qi.com | 116644.com | www.186212.com | www.674502.com | www.217210.com | www.109955.com | 77689.com | www.4400.tv | www.880694.com | www.gu67.com | www.408655.com | www.974782.com | 974585.com | www.567294.com | www.085535.com | 445408.com | www.718853.com | www.93116.cc | www.022494.com | 367808.com | 125063.com | www.dk78.com | www.579843.com | www.21917.cc | www.050024.com | www.950435.com | www.1580.org | www.185192.com | 950340.com | www.256891.com | www.36131.com | 027592.com | www.269057.com | www.367508.com | www.145758.com | h88m.com | 685027.com | 773323.com | 197656.com | hc45.cc | www.012125.com | www.971249.com | www.v53.com | www.529575.com | 973045.com | www.2st.com | www.062789.cc | www.808520.com | www.d54.xyz | 9498.cc | www.005798.com | www.8181.cn | 亿彩www.6832y.com | www.033962.com | 355194.com | 348099.com | www.838451.com | www.9481.me | www.3188.top | www.140255.com | 500彩票www.701496.com | www.4lm.com | www.0hl.com | www.58757.cc | www.021026.com | 233564.com | 023460.com | www.060145.com | www.626028.com | www.63or.com | www.26200.cc | www.31473.com | www.575836.com | www.128425.com | www.94lu.com | www.2583.cc | www.8200.biz | www.3977.live | www.04gq.com | www.pj03.cc | www.b69.cc | 六冠彩票www.liuguan000.com | 077220.com | 32577.cc | 655068.com | 083511.com | www.8669.cm | www.55250.com | www.552555.cc | www.30zp.com | 262330.com | www.ed6.cc | www.051905.com | www.78bg.com | www.dc53.com | www.343287.com | www.bl49.com | www.305960.com | www.569308.com | www.36713.com | 686337.com | www.204565.com | www.x2x6.com | 816832.com | 778051.com | www.14747.com | 099869.com | 53ba.com | 凤凰彩票www.88266d.com | www.38932.cc | www.4756.cc | www.3648.cc | www.000724.cc | www.758580.com | www.22295.cc | www.99272.cc | www.234333.com | www.973886.com | www.66870.com | www.857738.com | 971420.com | www.r11.cc | www.69820.com | www.256913.com | www.350034.com | www.198723.com | 241744.com | 211243.com | www.82836.cc | www.539658.com | 167279.com | www.103948.com | www.43586.com | www.96223.cc | www.092516.com | www.037716.com | www.19tz.com | 146829.com | 033620.com | 599946.com | 515473.com | www.1170.pw | www.220328.com | www.6876.vip | www.fq42.com | www.wx68.com | www.90920.com | 09118.cc | www.910371.com | 564885.com | www.cp0017.com | 733982.com | www.m66.top | 480025.com | 861262.com | www.87515.com | www.255527.com | www.237243.com | www.963331.com | www.860371.com | www.562117.com | www.1or.com | www.86885.com | www.822050.com | www.643813.com | www.kq03.com | www.90921.com | www.xw80.cc | www.026721.com | 366949.com | www.355341.com | www.827296.com | www.985056.com | www.994910.com | www.950480.com | www.658716.com | www.420654.com | www.258702.com | 048755.com | 368804.com | www.85815.cc | www.re07.com | www.173743.com | www.09ww.com | www.58122.com | www.cp5034.com | www.dg01.com | www.73nb.com | www.2966.org | www.966589.com | www.951757.com | www.494721.com | www.65uo.com | 293666.com | 福彩www.16878n.com | 280081.com | 070560.com | 746839.com | 734680.com | www.009631.com | www.99411.cc | www.525584.com | 317313.com | www.502722.com | www.84055.cc | www.93810.com | www.947209.com | 金冠彩票www.c4526.com | www.937756.com | www.976906.com | 3532.biz | www.85336.cc | www.wm78.com | 057290.com | www.64779.com | www.163978.com | www.370157.com | www.521477.com | 920287.com | www.84by.com | www.256629.com | www.20087.com | www.833032.com | 847282.com | www.17io.com | www.81151.com | www.779988.cc | www.23803.com | www.568441.com | www.315610.com | www.43kv.com | www.5528.in | www.lm55.com | www.85571.cc | www.965679.com | 356970.com | www.801311.com | 834230.com | www.87lq.com | www.838092.com | www.41ej.com | www.0973.date | www.32346.com | www.8828.live | 017602.com | www.kk63.com | 136042.com | 大福彩票www.df39.com | 253719.com | www.pp16.com | 275909.com | 梦想彩票www.33112k.com | 28001.com | www.000018.com | www.964174.com | www.6570.in | www.681519.com | www.313333.com | www.969682.com | www.3707.cc | www.640059.com | www.516723.com | www.695382.com | www.297878.com | www.262769.com | www.229606.com | www.862753.com | www.3kq.com | www.484967.com | www.264273.com | www.028921.com | 996670.com | 312960.com | www.759931.com | www.795259.com | www.873268.com | www.365227.cc | www.109828.com | www.21yb.com | www.yr8.com | www.lm91.com | www.04jo.com | www.46ru.com | www.kb33.com | www.661145.com | www.595705.com | www.0443.xyz | www.5472.com | www.832799.com | 86ut.com | 634811.com | 610395.com | www.820013.com | www.0039.com | www.072896.com | www.035318.com | www.162244.com | 353992.com | www.fx95.com | www.231322.cc | www.767909.com | www.629619.com | www.338164.com | www.177579.com | 众发彩票www.659zf.com | www.035455.com | www.062895.com | www.659234.com | www.455180.com | 028695.com | 110805.com | www.470012.com | www.661885.com | www.586839.com | www.515678.com | www.2373.cc | www.1800.tv | www.2448.net | 090046.com | www.713434.com | www.oo43.com | www.1291.vip | www.33009.cc | www.569581.com | www.081832.com | www.7109.net | www.666617.com | www.625766.com | www.619788.com | www.32ql.com | 860540.com | www.864759.com | www.625215.com | www.464268.com | www.39717.cc | www.022615.com | www.313980.com | 247750.com | www.310111.com | 大赢家彩票网www.178759.com | www.3600.org | www.56gj.com | www.6758.org | www.15rd.com | www.25359.cc | 576160.com | 947650.com | 大赢家彩票www.394211.com | 562031.com | www.543589.com | www.526950.com | www.959086.com | www.bu18.com | 242356.com | www.37885.cc | www.099026.com | www.eo25.com | www.u54.com | www.vh7.com | www.ka76.com | www.nm01.com | www.770749.com | www.063219.com | www.172.red | 23gy.com | 931400.com | www.68an.com | 458062.com | www.58nu.com | 931787.com | 98lc.cc | www.617573.com | www.8326.cc | 912051.com | www.cai3299.com | www.008594.com | www.fp19.com | www.14jf.com | www.26808.com | www.276345.com | www.9745.xyz | www.gb24.com | 860153.com | 544186.com | 0104.top | 金冠彩票www.49956j.com | www.b77.org | 十三国际www.596353.com | www.493003.com | www.228157.com | www.760302.com | 500彩票www.50024h.com | www.77536.cc | www.154833.com | www.45bf.com | www.233012.com | 484817.cc | 138996.com | 505147.com | www.gh42.com | 882520.com | yz04.cc | 972467.com | www.916648.com | 网易彩票www.505433.com | www.0889.cc | www.cd14.com | www.19ae.com | 128471.com | 917102.com | www.552952.com | 500彩票网www.61655t.com | www.589.cx | 亚投彩票www.ya515.com | 790809.com | www.977991.com | www.738516.com | www.a75.top | www.389609.com | www.069094.com | 102890.com | cai6262.com | www.256.org | www.hl69.com | www.wu11.com | www.197991.com | www.7747.cn | www.59322.cc | www.876477.com | www.269175.com | www.000549.com | www.597177.com | www.2139.com | www.vb1.com | www.188.com | www.20844.com | www.gt44.com | www.653656.com | 60245.com | www.078810.com | www.53119.cc | 759309.com | 963036.com | 162032.com | www.30594.com | www.032553.com | www.220036.com | www.160702.com | www.855616.com | www.cd65.com | 乐发彩票www.84577.com | 9hz.cc | www.7618.com | www.191977.com | www.072056.com | 36239.com | 788698.com | 520937.com | www.fn85.com | www.422342.com | 鸿运彩票www.hy2522.com | www.785409.com | www.79363.cc | www.b96.org | www.38875.com | www.3462.org | www.738028.com | www.375114.com | www.056388.com | www.75180.com | www.905363.com | www.496894.com | www.369319.com | www.97328.cc | www.456164.com | www.431276.com | 5618.me | 283751.com | 672488.com | www.25276.com | 星际www.m.55xj.vip | www.484950.com | www.909497.com | www.rg05.com | www.sc81.com | www.dv29.com | www.84966.com | www.93398.com | www.0236.me | www.360150.com | 791340.com | www.962472.com | www.572553.com | www.092158.com | www.72328.com | www.ib07.com | www.735665.com | www.092756.com | 362610.com | www.167774.com | www.543500.com | www.896516.com | www.59585.cc | www.513927.com | www.008600.com | www.1233.tv | www.09098.com | www.291653.com | www.258549.com | www.01501.com | 428722.com | www.60kl.com | www.751571.com | www.276499.com | www.162713.com | www.221919.com | www.630801.com | www.137255.com | www.83628.com | www.693258.com | www.515982.com | www.333902.com | www.sz7.com | www.108069.com | 739498.com | 359325.com | www.680613.com | www.905245.com | www.82xx.com | 048923.com | www.752228.com | 232389.com | www.91832.cc | www.2883.biz | www.120595.com | www.629369.com | www.598276.com | 430888.com | 339823.com | www.02360.cc | www.370849.com | www.935600.com | www.518.net | www.513678.com | qw66.cc | www.502939.com | www.426011.com | 512053.cc | www.404358.com | www.027963.com | www.67nq.com | www.69657.com | www.81sg.com | www.3636.hk | www.978142.com | 137446.com | www.160755.com | www.89549.com | ks4.com--ks4.com | www.821715.com | www.925862.com | www.77876.com | www.68az.com | www.7358.biz | www.tt77.cc | www.077991.cc | www.954508.com | www.634104.com | www.307170.com | 91彩票www.9155b.com | www.be77.com | www.904150.com | www.170681.com | www.911171.com | www.721127.cc | www.860987.com | www.563281.com | www.2344.vip | www.286961.com | www.210737.com | www.025197.com | www.48278.com | www.2144.online | www.pu72.com | 438722.com | 361635.com | 342024.com | 49tj.com | 939621.com | 270305.com | www.964796.com | www.807519.com | 394885.com | www.981497.com | www.4137.cc | www.887469.com | www.61257.cc | www.395651.com | 963024.com | 06nz.com | 671480.com | 500彩票www.501346.com | www.299027.com | www.571708.com | www.0599.link | 惠民彩票www.19kpl.com | 136130.com | www.087977.com | www.179187.com | www.584522.com | www.xv1.com | 482903.com | rp75.com | 500彩票www.66653h.com | www.836326.com | 大赢家彩票平台www.817055.com | www.763078.com | www.254060.com | 384050.com | www.062432.com | www.23763.cc | www.766028.com | www.589322.com | www.903802.com | www.452825.com | 353123.com | www.159774.com | www.585733.com | 500万彩票www.500yf.com | www.914646.com | www.776144.com | www.585712.com | www.053786.com | www.870438.com | www.669088.com | 610075.com | www.42ya.com | www.448996.com | www.209032.com | 221080.com | www.620356.com | www.126342.com | 52416.cc | 801742.com | www.32636.com | 凤凰彩票www.77802w.com | 购彩票www.c5235.com | www.0774.cn | www.237440.com | www.284928.com | www.06tt.com | www.001144.cc | www.348355.com | www.708936.com | www.677553.com | www.515813.com | www.262444.com | 159501.com | www.158379.com | www.510004.com | www.257617.com | www.269223.com | www.066781.com | www.770438.com | www.670585.com | www.522697.com | www.7736.in | www.907378.com | www.718231.com | 373814.com | 557019.com | www.440169.com | 53ud.com | www.rm64.com | www.01ea.com | www.8qh.com | www.312811.com | 573470.cc | www.586026.com | www.485602.com | www.873810.com | www.966354.com | 794848.com | 978420.com | 900834.com | www.253957.com | www.188422.com | www.283997.com | 443993.com | www.2521.cc | www.292.club | www.8288.live | 豪彩VIPwww.946854.com | www.078106.com | www.671972.com | www.558985.com | www.763477.com | www.658214.com | www.176921.com | 954817.com | 340093.com | www.39943.com | www.1297.cm | 976874.com | www.66ws.cc | www.ef62.com | www.640889.com | www.016127.com | 386920.com | www.636.hk | www.209035.com | www.8181.vip | www.618118.com | www.016466.com | www.074791.com | www.128041.com | www.37317.cc | www.7038.cm | www.755937.com | www.356906.com | www.960743.com | www.ub71.com | www.633222.com | www.612095.com | www.713132.com | www.916634.com | www.834811.com | www.213772.com | www.ys3.cc | 986793.com | 243938.com | www.365910.cc | www.427959.com | www.89184.com | www.94mo.com | www.109928.com | www.797676.cc | www.0687.org | www.44605.com | www.07684.com | www.77549.com | www.724933.com | www.7080.in | www.22ep.com | www.796542.com | www.972605.com | www.874600.com | www.127462.com | www.245234.com | www.216970.com | www.463619.com | www.027011.com | www.92484.com | www.919877.com | www.dd.cc | www.fi5.com | www.81223.com | www.8032.top | www.1998.online | www.so9.com | www.0010.pw | 13e彩票www.510860.com | zv33.com | www.68695.cc | 大赢家彩票平台www.927320.com | www.p29.com | www.252664.com | 易盈彩票www.7793x.com | 福彩www.86267d.com | www.627068.com | www.05202.com | www.1913.top | www.240450.com | 143618.com | 343224.com | www.048174.com | www.035665.com | 870353.com | www.989430.com | www.581848.com | www.741338.com | www.913016.com | 105662.com | 006457.com | www.107948.com | www.731646.com | www.474949.com | www.690352.com | www.7161.top | www.223502.com | www.4139.biz | www.88ke.cc | www.060538.com | www.836181.com | www.678418.com | www.974862.com | www.78830.com | www.879703.com | www.33751.cc | www.2563.vip | www.503939.com | 088877.com | 025611.com | www.33650.com | www.574150.cc | www.ps07.com | www.254008.com | www.854483.com | 982043.com | www.9420.mobi | tq67.com | www.618088.com | www.786252.com | www.200833.com | 609094.com | www.054567.com | www.4531.cm | www.01qf.com | 545234.com | 051026.com | www.we78.cc | www.69zh.com | www.279657.com | www.52577.cc | www.380106.com | www.161164.com | www.390095.com | www.130476.com | www.927700.com | www.vr95.com | www.48611.com | 536729.com | www.1847.press | www.552257.com | www.519817.com | www.736571.com | www.0744.org | www.64pt.com | www.50865.com | www.281232.com | www.126902.com | www.yo95.com | yz36.com | 吉彩www.602327.com | www.251078.com | www.682300.com | www.363196.com | www.633644.cc | www.123213.com | www.190056.com | www.079161.com | www.14735.com | www.16081.com | 702285.com | www.hz27.com | 964157.com | www.805659.com | 13bm.cc | www.226015.com | www.149300.com | 928012.com | www.013995.com | www.461377.com | www.834.net | www.16978.com | 56zr.com | www.130.red | www.301352.com | www.lz03.com | www.375244.com | 733916.com | 7098.biz | www.2285.net | www.181815.com | www.9434.net | www.312038.com | 12ut.com | www.27186.cc | www.382508.com | www.151169.com | 966809.com | www.318792.com | www.k88.in | www.8826.wang | www.4881.biz | www.24zi.com | www.323247.com | www.563708.com | www.634914.com | 173151.com | www.200187.cc | www.468105.com | www.245026.com | pv04.com | www.570284.com | 556935.com | 025324.com | www.54ir.com | www.670089.cc | www.001802.com | www.472148.com | www.46053.cc | www.539507.com | www.88575.cc | www.581073.com | www.15km.com | 398234.com | www.909930.com | www.941166.com | www.741618.com | www.mm44.cc | 930562.com | 775009.com | 076957.com | 668314.com | 500万彩票www.39500o.com | 406823.com | www.57381.cc | www.806393.com | www.203474.com | www.168961.com | yh61.cc | www.85xk.com | 003339.com | www.800678.com | www.a04.com | 幸运彩票www.044592.com | www.60428.com | www.312220.com | www.963007.com | www.ca56.com | 753888.com | www.616622.com | www.323367.com | www.648268.com | www.209023.com | 339882.com | www.966341.com | www.961605.com | www.283637.com | 旺旺彩票www.938849.com | 趣彩彩票www.c177.com | www.036558.com | www.430420.com | www.1663.me | www.4175.cc | www.293345.com | www.012140.com | www.83442.com | www.217267.com | www.160071.com | www.287356.com | 129924.com | www.9281.shop | www.029210.com | www.6259.biz | 664678.com--29149.com | www.176836.com | www.533441.com | 019199.com | www.130609.com | www.3ai.cc | www.942566.com | www.085526.com | 518308.com | www.836767.com | 599818.com | www.871629.com | 583086.com | www.697676.cc | www.4960.com | www.16118.com | www.028276.com | www.0097.cm | www.07787.com | www.533608.com | 463069.com | www.456338.com | www.483807.com | www.8898.mobi | www.969595.com | www.432995.com | www.799085.com | www.008550.com | www.882697.com | 769026.com | 宏发网www.170955.com | www.007926.com | www.cp8466.com | 896481.com | www.9230.top | www.xf97.com | cai996.cc | www.857798.com | www.967597.com | www.396427.com | www.22703.com | www.nz25.com | 984071.com | www.069815.com | www.n11.cm | www.0180.top | 579436.com | 198079.com | www.590228.com | 241149.com | www.cp106.cc | 356374.com | 大赢家彩票www.546411.com | 大赢家彩票平台www.935257.com | www.922058.com | www.6011.biz | www.7444.xyz | 428198.com | www.055945.cc | www.693.in | www.511819.com | www.432132.com | www.480220.com | www.178663.com | www.433866.com | www.493628.com | www.99848.com | 590877.com | www.857548.com | www.dl88.cc | www.176090.com | www.150896.com | www.369140.com | www.664985.com | www.981715.com | www.674696.com | www.023171.com | www.91pk.com | 030029.com | www.357255.com | www.358667.com | 56730.com | www.1139.vip | www.198298.com | www.116308.com | 364989.com | www.920734.com | www.474125.com | www.116335.com | www.919019.com | www.835233.com | 479654.com | 99432.com | 033714.com | www.pp77.cc | www.094155.com | www.256234.com | www.926058.com | 950547.com | www.608291.com | 028467.com | www.429738.com | www.089583.com | www.062396.com | www.441182.com | www.6321.cm | www.ca4.cc | www.839924.com | www.680928.com | 3068.biz | www.id46.com | www.01.me | 973726.com | 爱购彩票www.413552.com | 679105.com | www.66648.com | www.sv78.com | 523506.com | www.930691.com | www.2336.pw | www.os83.com | www.789944.com | 811049.com | www.778811.com | www.182863.com | www.99356.cc | 191495.com | www.377010.com | 529313.com | www.hl3.com | 5713.biz | www.714388.com | www.401001.com | www.066643.com | 552398.com | www.8854.vip | www.365850.cc | www.vt9.com | 378926.com | 271678.com | www.97aj.com | www.cp2.cc | 499888.com | 443881.com | www.397502.com | www.652.website | www.947929.com | www.712930.com | www.837365.com | www.712517.com | www.923478.com | www.512775.com | www.571455.com | www.719582.com | www.518278.com | www.63759.cc | www.121020.com | www.804166.com | s78.top | 68彩票www.68689m.com | www.yl44.com | www.cp342.com | www.8273.biz | www.082688.com | 006156.com | www.657964.com | 574119.com | www.810902.com | s65.cc | 943336.com | www.736152.com | www.468736.com | www.056061.com | www.1152.net | 500彩票网www.658770.com | 024706.com | www.654498.com | www.58559.cc | www.367836.com | www.35262.cc | www.an25.com | 896000.com | 10345.cc | www.986569.com | www.62no.com | www.049876.cc | www.zp39.com | www.63382.cc | www.67997.com | www.088970.com | www.47471.com | www.033609.com | www.ma02.com | www.921180.com | www.5550.in | www.805781.com | 558405.com | 792305.com | 708705.com | www.927608.com | www.397134.com | www.271644.com | www.11xj.cc | www.152227.com | www.152895.com | www.mo49.com | www.220031.com | 549177.com | www.53685.cc | www.179986.com | www.18055.cc | www.799499.com | 322571.com | www.133054.com | www.6429.com | 761655.com | www.896530.com | www.884575.com | 350587.com | www.908568.com | www.319061.com | www.984826.com | www.13225.com | 902896.com | 870491.com | www.qy90.com | www.84006.com | www.20qs.com | www.826500.com | 608948.com | 955242.com | 986983.com | 517347.com | www.744854.com | www.575889.com | www.w74.club | www.972981.com | www.711800.com | www.366103.com | www.487866.com | www.99736.cc | www.xb99.cc | www.34290.com | www.01001.cc | www.41jm.com | www.go11.com | ag71.cc | www.197936.com | www.881401.com | www.972794.com | www.987267.com | www.927225.com | 671660.com | 059944.com | 791412.com | www.980176.com | www.662955.com | 097279.com | www.758309.com | www.240786.com | www.875254.com | www.399119.com | www.921819.com | www.986464.com | www.qr13.com | 870969.com | www.732639.com | www.1809.vip | www.203023.com | www.257166.com | www.28nf.com | www.085265.com | www.82494.com | 790575.com | www.32mt.com | www.99je.com | www.731419.com | www.808907.com | www.850204.com | www.34412.com | 023553.com | www.198.bid | www.31yo.com | www.855038.com | www.7479.me | www.70144.com | www.3166.org | 975448.com | www.ft10.com | 018465.com | 983236.com | 007880.com | E彩堂www.43818b.com | 953760.com | www.fe67.com | www.208293.com | www.926603.com | 124477.com | 538579.com | www.84842.cc | www.8210.org | www.345683.com | www.692999.com | www.000506.com | www.34hd.com | www.25919.cc | 338074.com | www.827118.com | www.8yb.cc | www.91fl.cc | www.31wt.com | www.79ps.com | www.cp9859.com | www.46279.com | www.916227.com | www.622202.com | www.81dd.com | www.60121.com | www.zr1.com | www.084656.com | www.719502.com | www.497097.com | 71oh.com | 大赢家彩票平台www.179223.com | www.657683.com | www.119535.com | www.62620.cc | www.122163.com | www.122429.com | www.191696.com | www.5169.online | www.869915.com | www.262519.com | www.027754.com | www.122613.com | www.856873.com | www.639780.com | www.401819.com | www.144221.com | www.51008.com | www.336150.com | 979354.com | www.655527.com | www.754306.com | www.029321.com | www.b04.top | www.297808.com | 972907.com | www.954846.com | www.543265.com | www.82029.com | www.5771.com | www.01130.cc | www.0708.wang | www.98mz.com | www.mw1.com | www.2571.win | www.56569.com | www.yw79.com | 97ql.com | PK彩票www.700724.com | www.927131.com | www.630599.com | www.153441.com | www.165365.cc | 332738.com | www.728358.com | www.77103.com | www.7116.live | www.0474.date | www.fp0.com | www.743438.com | www.53ib.com | www.92rz.com | 307982.com | www.951584.com | www.958760.com | www.487836.com | www.5752.top | www.xn08.com | www.40628.com | 107586.com | www.101564.com | www.693571.com | www.22485.com | www.461766.com | www.266885.com | www.017668.com | www.3tt.cc | www.22452.com | www.603163.com | www.655238.com | www.439626.com | www.023847.com | www.0488.top | www.108937.com | www.287033.com | www.x97.com | www.y8.cc | www.645310.com | www.947247.com | www.576486.com | 亿龍彩票www.1368h.cc | 293303.com | www.732693.com | www.12ni.com | www.188405.com | www.181395.com | www.22523.com | www.9499.cm | 449226.com | www.05di.com | www.521035.com | www.968453.com | 448117.com | 572510.com | 010539.com | ng43.com | www.023380.com | www.995705.com | www.7004.vip | www.874934.com | www.w22.xyz | 896883.com | www.5676.com | www.89345.com | www.90ue.com | www.62100.com | www.913507.com | www.811730.com | www.885753.com | 56867.com | www.533307.com | 404898.com | www.620318.com | www.739742.com | www.46tq.com | www.949609.com | 668720.com | www.664736.com | www.299505.com | www.vb10.com | 977475.com | www.811612.com | www.989410.com | www.554301.com | www.345260.com | www.20204.com | www.787577.com | www.833683.com | www.433350.com | www.782900.com | www.830505.com | www.ne47.com | www.966784.com | www.698641.com | www.bo32.com | www.942784.com | www.94666.cc | www.8889.biz | www.024234.com | www.9972.top | www.27445.com | www.cu37.com | 826973.com | www.231753.com | www.365528.cc | www.718903.com | www.028319.com | www.618383.cc | www.301744.com | www.19891.com | www.55949.cc | www.989297.com | www.407203.com | www.904058.com | 160275.com | www.538909.com | 418009.com | www.611554.com | www.cai39.cc | 220485.com | www.592273.com | www.951325.com | 139858.com | www.676631.com | www.889333.com | www.235372.com | www.182388.com | www.336505.com | www.835025.com | www.753875.com | www.3547.cc | 567324.com | www.234145.com | www.315920.com | www.ip33.com | www.740622.com | www.423722.com | www.482.in | www.886310.com | www.538380.com | www.119366.com | www.260358.com | 678244.com | www.984536.com | www.259185.com | www.096360.com | www.713806.com | www.596220.com | www.042058.com | 天天彩票www.106276.com | www.01804.com | www.903317.com | www.0492.cc | www.29ck.com | www.590300.com | www.359955.com | www.1936.vip | www.202327.com | www.30fq.com | www.242867.com | 171017.com | 336618.com | www.730611.com | www.22732.com | www.723455.com | 223459.com | www.922652.com | www.1261.xyz | 359900.com | 520908.com | www.33vh.com | 110657.com | www.332274.com | 网易彩票www.077wy.com | www.262444.com | www.43483.com | 362139.com | www.773819.com | 751287.cc | 新盈彩www.xinyc2.com | www.893388.com | www.850655.com | www.787968.com | www.232956.com | 195817.com | www.49hp.com | 780015.com | www.105483.com | www.330963.com | www.192684.com | www.617828.com | www.318587.com | 927540.com | www.283536.com | 43191.com | www.2392.win | www.91331.cc | www.cp6552.com | www.37869.cc | www.279508.com | www.8896.vip | 78ha.com | j52.me | 328764.com | www.288811.cc | 645368.com | www.568176.com | www.cai9488.com | www.qt06.com | 977595.com | www.237111.com | 966709.com | www.004947.com | www.0647.net | www.131336.com | www.5881.top | 5003.vip | www.835921.com | 687002.com | www.699073.com | www.884818.com | www.cp781.com | www.767516.com | www.7608.top | 526230.com | www.714769.com | www.995139.com | www.374037.com | 130165.com | 227448.com | 636439.com | www.947525.com | www.282899.com | www.5400.vip | 282997.com | www.1270.wang | www.hm00.com | yz03.com | www.634197.com | www.573480.cc | www.000943.com | 体彩天下www.tctx6.com | www.001667.com | www.267297.com | 556208.com | www.5457.pw | www.984178.com | www.285542.com | www.233416.com | www.05053.com | 554659.com | www.rh65.com | www.bx70.com | www.018000.com | www.569179.com | www.900717.com | 175289.com | www.850663.com | www.737876.com | www.619489.com | www.013488.com | 汇彩网www.www.hcw266.com | 190963.com | www.828800.com | www.69as.com | www.011095.com | www.y10.org | 899847.com | www.773967.com | 731465.com | 068379.com | 015834.com | www.447336.com | www.41888.cc | 299380.com | 200547.com | www.30485.com | 775348.com | www.563907.com | www.54ct.com | www.92eu.com | www.633909.com | www.58715.cc | 535157.com | 173460.com | www.033640.com | www.259742.com | www.317757.com | www.689072.com | www.085266.com | www.450069.com | 彩宝www.911888aa.com | www.232787.com | www.1649.vip | www.2117.win | 873411.com | 13pj.cc | www.977647.com | www.900734.com | www.469809.com | 奔驰彩票www.29178f.com | www.155229.com | www.4283.vip | 500万彩票www.39500l.com | 08kp.com | www.463665.com | www.029964.com | www.228988.com | www.211057.com | www.203131.com | www.76891.com | www.93685.cc | www.pf21.com | www.63oc.com | 801022.com | www.597334.com | 979983.com | www.798662.com | www.618074.com | www.gg75.com | www.714238.com | www.07va.com | www.134666.com | www.36430.com | www.91365.com | www.615069.com | www.486726.com | www.83zv.com | www.042896.com | www.300181.com | www.5168.club | www.539368.com | www.143544.com | www.698941.com | www.389059.com | www.795598.com | www.k44.me | 大玩家彩票www.84499m.com | www.639513.com | www.206065.com | www.555.red | www.1138.in | www.563177.com | www.mz36.com | www.567132.com | www.829077.com | www.565397.com | www.091307.com | www.783799.com | 019146.com | www.121873.com | 8077.cc | www.158715.com | 500彩票www.547077.com | www.310279.com | 369404.com | www.552559.com | www.804171.com | www.1352.cn | www.093549.com | www.698437.com | www.437705.com | www.030076.com | www.ch3.com | 500彩票网www.61655y.com | www.885050.com | www.527666.com | www.71142.com | www.97736.cc | www.dn69.com | 129854.com | www.74235.com | 350587.com | www.085073.com | www.973480.com | www.658338.com | www.059910.com | www.8673.me | www.646264.com | www.53129.cc | 623083.com | www.sg60.com | www.919061.com | www.974086.com | www.874303.com | www.225887.com | www.5439.vip | www.255825.com | www.0775.xyz | www.sy12.cc | www.967475.com | 752110.com | www.738183.com | www.586042.com | www.777174.com | www.51653.com | www.nh04.com | 365504.cc | www.566012.com | www.997973.com | www.184351.com | www.11uh.com | 747990.com | 764233.com | www.77603.com | www.620101.com | www.320258.com | www.ra36.com | 976740.com | www.0hl.com | www.889715.com | www.46ul.com | www.22151.cc | www.903632.com | www.969471.com | www.123490.com | www.651208.com | www.382199.com | www.it1.com | www.19wg.com | www.506832.com | www.871654.com | 520.red | 864805.com | 414110.com | www.28176.com | www.350651.com | www.mf36.com | www.711650.com | www.848513.com | www.146488.com | 153376.com | www.94789.cc | www.885664.com | www.43yo.com | www.695352.com | 620595.com | www.739282.com | www.110409.com | www.800524.com | www.690944.com | www.891087.com | 539701.com | 01769.com | www.733769.com | www.217822.com | 804606.com | www.805037.com | www.863029.com | www.2636.cc | 全民乐彩票www.2934m.com | www.955934.com | www.141665.com | www.0058.loan | www.858314.com | www.864609.com | www.200045.com | www.1567.top | www.13w.com | www.190106.com | www.376826.com | www.371022.com | www.88262.com | www.509078.com | 145544.com | www.277011.com | 670901.com | 615283.com | www.810380.com | www.048858.com | www.25tj.com | www.911038.com | www.027956.com | www.286873.com | www.iw05.com | 87881.com | www.r79.xyz | 爱购彩票www.3552p.com | www.d28.hk | www.14pe.com | www.947536.com | www.206068.com | www.12989.cc | www.04oi.com | 761224.com | www.8125.top | www.600952.com | www.im74.com | www.121334.com | www.013673.com | 783663.com | www.970553.com | www.476250.com | www.08689.com | 32we.com | www.613311.com | www.502975.com | www.28396.cc | 955643.com | www.79557.cc | www.666587.com | 4377.biz | www.333560.com | www.83173.com | www.542809.cc | www.205899.com | 003742.com | www.970208.com | www.493787.com | www.163367.com | www.365205.cc | 590155.com | www.117309.com | www.bn21.com | 福利彩票www.78700f.com | www.752303.com | www.969669.com | www.ua82.com | 870448.com | 309290.com | 438107.com | www.67393.com | 963407.com | www.816099.com | www.111744.com | www.127145.com | 987616.com | www.176773.com | www.311832.com | www.79dj.com | 467007.com | 236568.com | 431558.com | www.042244.com | www.851884.com | www.690001.com | www.151028.com | 651020.com | www.974895.com | www.139244.com | 红鹰彩票www.hy6932.com | 61828.com | 295432.com | www.659666.cc | www.910799.com | www.076111.com | www.88735.com | 500彩票网www.55220.com | www.45054.com | 567141.com | www.760395.com | www.8191.biz | 84292.com | www.556546.com | www.800115.com | www.917767.com | www.255121.com | www.85oj.com | www.6036.vip | www.5863.cc | www.962994.com | 932244.com | www.ea74.com | www.621867.com | www.01073.com | www.cc7.cc | www.248677.com | 316051.com | www.383467.com | 803329.com | www.298388.com | www.898289.com | 500彩票网www.65707u.com | 023472.com | 559639.com | 902946.com | www.651398.com | www.036649.com | www.115987.com | 500彩票www.26299q.com | 974083.com | www.622264.com | 640059.com | www.660118.com | www.672308.com | 624758.com | www.373132.com | www.271521.com | www.46420.com | www.635058.com | 158414.com | 537333.com | www.358215.com | www.6646.cn | www.fz87.com | www.76rc.com | 开心彩票www.ck5568.com | 075976.com | www.97218.cc | 095708.com | www.52500.cc | www.5088.me | www.876055.com | 657093.com | www.434790.com | 484228.com | www.380504.com | www.318975.com | www.h65.com | www.246129.com | 999671.com | www.915368.com | 057821.com | www.297626.com | www.520401.com | www.079657.com | 天玺彩票www.308550.com | www.us63.com | www.8891.net | GO彩www.ban03.com | www.502264.com | 332334.com | 757329.com | www.926621.com | www.745522.com | www.374244.com | 308363.com | www.829044.com | cm52.com | 中彩网www.61233f.com | www.3658.in | 850818.com | 吉利彩票www.66376z.com | www.51na.com | www.63655.cc | www.590378.com | www.139830.com | www.087870.com | www.2025.org | 彩客网www.011225.com | www.729965.com | www.757890.com | www.594067.com | www.677006.com | www.761141.com | www.559547.com | www.913627.com | www.286033.com | www.795702.com | www.088752.com | www.sb73.com | www.0778.cm | www.93es.com | www.157.pw | 156482.com | 113403.com | www.338427.com | 974724.com | 804576.com | 964482.com | www.f81.net | www.706928.com | 98299.com | www.305092.com | www.287293.com | 220863.com | www.559908.com | www.423887.com | 577013.com | www.762694.com | www.386411.com | www.87iz.com | www.415.in | www.9721.club | www.400633.com | www.4477.tv | www.83as.com | www.333736.com | www.cai1188.com | www.391938.com | www.14aj.com | www.193600.com | 758977.com | www.693351.com | 302576.com | www.587207.com | www.262686.com | www.033046.com | www.nd1.com | www.960938.com | www.90eg.com | www.638713.com | www.852876.com | www.2mj.cc | www.069031.com | www.300029.com | www.460579.com | www.30197.com | www.162964.com | www.0098.wang | 958301.com | www.930693.com | www.595399.com | www.334427.com | 126472.com | www.000345.cc | www.672661.com | www.507152.com | www.5856.mobi | 377692.com | www.457678.com | www.27129.cc | www.0731.pro | www.753365.com | www.874692.com | www.501809.com | www.903667.com | www.568036.com | www.035911.com | www.781.date | www.888058.com | www.53wy.cc | www.886557.com | www.47pv.com | www.448484.com | www.8131.cn | www.068336.com | 122315.com | www.8944.tv | 639204.com | www.635166.com | www.457543.com | www.3730.org | 399533.com | www.539483.com | www.80bo.com | 008953.com | 好运彩www.725106.com | www.rt04.com | www.495228.com | www.767222.com | www.558513.com | www.674521.cc | www.845944.com | 153487.com | www.qr19.com | www.8jh.cc | www.882999.com | www.017957.com | 968240.com | www.441777.com | www.730281.com | www.823440.com | www.407177.com | www.060612.com | www.338893.com | VIP彩票www.508533.com | 180729.com | 865140.com | 购彩票www.c5236.com | www.194002.com | www.460021.com | www.73561.cc | www.vi11.cc | www.024074.com | www.44548.com | xl48.com | 519276.com | 036656.com | www.894784.com | www.7031.cn | 16彩票www.331616a.com | www.365121.cc | 454250.com | 006423.com | www.596541.com | www.129318.com | www.511211.com | www.404000.cc | 026857.com | www.56uc.com | 幸运彩票www.768299.com | www.884125.com | www.604409.com | www.06800.com | www.021149.com | www.zv89.com | www.708578.com | www.67kx.com | 500彩票www.51515a.com | www.tl75.com | www.89249.com | www.11675.cc | 174868.com | www.r80.top | www.733311.com | www.0633.win | www.040886.com | www.64966.cc | www.96961.com | www.164529.com | www.056562.com | www.dk8.com | 040116.com | www.7375.pw | www.809322.com | www.084677.com | 702716.com | www.pe80.cc | www.884050.com | www.924178.com | www.322897.com | www.39867.cc | 公益福彩www.gyfc2.com | www.128371.com | www.903692.com | www.686980.com | www.160944.com | 86312.com | www.090028.com | www.110301.com | www.168789.cc | www.9518.xyz | www.cai8077.com | www.567289.com | cp463.com | www.92887.com | www.957574.com | www.1831.bid | www.821398.com | www.432986.com | 全民乐彩票www.2934l.com | 凤凰彩票www.77802p.com | www.863219.com | www.663455.com | www.022728.com | www.53kj.cc | 016543.com | www.610535.com | www.170515.com | www.237198.com | www.kq84.com | www.259062.com | www.7608.cn | 506830.com | www.33153.com | 易彩网www.36166x.com | www.pa01.com | www.271058.com | www.mc64.com | www.84.cc | www.134446.com | www.62ju.com | www.68651.cc | 245368.com | 659306.com | www.529310.com | www.720408.com | www.33353.cc | www.331351.com | www.989914.com | www.735708.com | www.920120.com | www.06ug.com | www.fg59.com | www.729701.com | www.947356.com | www.094799.com | 962649.com | www.761477.com | www.927003.com | www.97522.cc | www.yi74.com | www.862025.com | 025894.com | www.4666.cn | www.35572.cc | www.280190.com | www.26799.cc | www.aa89.com | www.804877.com | www.557477.com | www.082622.com | 0048.cc | 751523.com | www.556685.com | www.600545.com | 120699.com | www.842488.com | www.2300.cc | www.nc79.com | www.790318.com | www.008509.com | www.638765.com | www.730909.com | www.795295.com | www.323727.com | www.141785.com | www.692189.com | www.6225.me | www.jb44.com | www.23py.com | www.557638.com | www.15bc.com | 974369.com | www.949499.com | 796421.com | www.470083.com | www.q03.space | www.943448.com | www.070722.com | www.004713.com | 657072.com | www.823435.com | www.190027.com | 3668彩票www.3668o.com | www.458620.com | www.nq53.com | www.786018.com | www.7125.me | www.31oz.com | 095858.com | www.728899.com | www.188293.com | www.176561.com | www.296770.com | bv18.com | www.539976.com | www.035517.com | www.ux50.com | www.486787.com | www.gb12.cc | www.2651.net | www.110385.com | www.cp651.com | www.811753.com | www.52662.cc | 894839.com | www.939941.com | www.95gf.com | www.923197.com | www.927985.com | www.474147.com | www.395785.com | www.26153.cc | 570226.com | www.622244.com | www.6200.wang | www.92uq.com | www.911016.com | www.72251.com | www.259657.com | www.df71.com | www.819367.com | www.090063.com | 638012.com | 948621.com | www.642789.com | www.130580.com | www.332.live |